Synthetic Spatiotemporal Plasmonic Vortices On Chip

in: arXiv (2025)
Chen, Qian; Zhang, Shuoshuo; Xian, Guoyu; Hu, Haoqiang; Wu, Xiaohua; Wu, Xiaofei; Huang, Jer-Shing; Huang, Chen-Bin; Zhang, Yuquan; Yuan, Xiaocong; Min, Changjun; Dai, Yanan
Spatiotemporal vortices are polychromatic modes that intertwine orbital angular momentum (OAM) in space and time. Here we introduce a new class of such vortices, spatiotemporal plasmonic vortices (STPVs), carrying nontrivial topological spin textures. They are generated by chronotopic interference of temporally delayed plasmonic eigen-vortices, where a -phase dislocation in the space-frequency domain maps into a 2 spiraling phase in space-time, with the resulting focus-defocus dynamics emulate U(1) gauge transitions. Using interferometric time-resolved photoemission electron microscopy (ITR-PEEM), we directly image their nanometer-attosecond (nano-atto) evolution and control vortex number and position. Quantum-path analysis of coherent two-photon photoemission (2PP) processes reveals the nonlinear plasmonic polarization fields and angular-momentum conservation, establishing STPVs as a platform for probing spatiotemporally structured quantum matter

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