Compact high-repetition-rate source of coherent 100 eV radiation

in: Nature Photonics (2013)
Pupeza, Ioachim; Holzberger, Simon; Eidam, Tino; Carstens, Henning; Esser, Dominik; Weitenberg, Johannes; Rußbüldt, Peter; Rauschenberger, Jens; Limpert, Jens; Udem, Thomas; Tünnermann, Andreas; Hänsch, Theodor W.; Apolonski, Alexander; Krausz, Ferenc; Fill, Ernst
Coherently enhancing laser pulses in a passive cavity provides ideal conditions for high-order harmonic generation in a gas, with repetition rates around 100 MHz (refs 1–3). Recently, extreme-ultraviolet radiation with photon energies of up to 30 eV was obtained, which is sufficiently bright for direct frequency-comb spectroscopy at 20 eV (ref. 4). Here, we identify a route to scaling these radiation sources to higher photon energies.We demonstrate that the ionization-limited attainable intracavity peak intensity increases with decreasing pulse duration. By enhancing nonlinearly compressed pulses of an Yb-based laser and coupling out the harmonics through a pierced cavity mirror, we generate spatially coherent 108 eV (11.45 nm) radiation at 78 MHz. Exploiting the full potential of the demonstrated techniques will afford high-photon-flux ultrashort-pulsed extreme-ultraviolet sources for a number of applications in science and technology, including photoelectron spectroscopy, coincidence spectroscopy with femtosecond to attosecond resolution5,6 and characterization of components and materials for nanolithography7.

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